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Say that Sho did join chronos. What do you think would have happened to him? I think he would have been tested on like Lisker, but after that.....

The reason they did not is because it is an unacceptable risk. We only saw Acids used when zoanoids broke into the Relic, we do not know if it would take a more drastic measure on detecting a more powerful creature inside though this is possibly unlikely due to the fact a zoanoid managed to get inside and out of the relic thanks to large numbers of them trying. Though it did pay for that with it's life, again not something a zoalord would view as a resounding success. Also the main reason they never did has being hinded in the manga. when Guyot attacked Guyver 3 and the team directly Hamical didn't react well calling the move rash and not the norm. If a zoalord tried to risk himself doing what you suggest chances are he'd be shot down by command due to the risk of not only the zoalords life but more so to the zoa-crystal itself.

I doubt a Creator ship could stop him... they have not displayed anything capable of stopping a Zoalord. Kind of weird that they sent Zoanoids inside when any of the Zoalords could just have forced their way in and, protected by their force shield, look around at their leisure. Perhaps they were afraid there could be surprises inside they were not prepared for.

Guyot would have used the Remover on him as soon as he worked out how to activate it. That was only a matter of time. That way, he might even have beaten Archanfel to the punch. Sho might even be the better for it. After Guyot removes the armor, only human Sho would be left. I bet even the communication nodes on his back would disappear like scar tissue. Would Guyot let him live? I think he would. He would be so over the moon with having the unit, he might even be grateful. Of course, the question is whether it would do Sho any good in the long term... I wonder if Guyot, merged with the unit, would have been more powerful than Archanfel. Probably pretty close.