To lace the with adamantium, would post a few too many problems.
While yes, it would be the most durable armor, movement, retraction, or summoning would be a problem due to the bonding process being very
un-selective in what it bonds to.
Wolverine's case was they pumped him full of nanites to make sure his bones would still produce marrow and blood. Then with an arse load (hundreds in one bone's area) of needles they pump him full of molten adamantium (over 1000 degrees worth of hot metal), basically him, the water, and anything else wet boiled nicely.
If you produced billions of nanites made of adamantium, maybe.